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Battery degradation evaluation based on impedance spectra using a limited number of voltage-capacity curves
School of Mechanical Engineering, Beijing Institute of Technology, No. 5 South Zhongguancun Street, Haidian District, Beijing, 100081, China.
School of Mechanical Engineering, Beijing Institute of Technology, No. 5 South Zhongguancun Street, Haidian District, Beijing, 100081, China.
Contemporary Amperex Technology Co.Limited, Ningde, 352106, China.
School of Mechanical Engineering, Beijing Institute of Technology, No. 5 South Zhongguancun Street, Haidian District, Beijing, 100081, China.
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2024 (English)In: eTransporation, E-ISSN 2590-1168, Vol. 22, article id 100347Article in journal (Refereed) Published
Abstract [en]

Degradation prediction is crucial for ensuring safe and reliable operation of batteries. However, relying solely on capacity to characterize aging cannot comprehensively represent the health status of the battery. This work explores the potential of using a limited number of partial voltage-capacity curves to evaluate battery degradation with the aid of deep learning approaches, which can be used for onboard applications. A sequence-to-sequence model is proposed to predict the electrochemical impedance spectra during battery degradation. It only uses capacity sequences within a specific voltage range at fixed voltage increments from a limited number of cycles, which can be flexibly adapted to different life stages in an end-to-end manner. The proposed method has been validated based on the developed degradation dataset. The root mean square errors for the prediction of impedance spectra are less than 1.48 mΩ. Capacities and resistances associated with electrochemical processes can be further extracted from the obtained impedance spectra, facilitating a comprehensive evaluation of battery degradation. As a limited number of measured data are needed, the proposed method can reduce data storage requirements and computational demands, which enables fast and comprehensive aging diagnosis.

Place, publisher, year, edition, pages
Elsevier, 2024. Vol. 22, article id 100347
Keywords [en]
Aging diagnosis, Battery degradation, Deep learning, Impedance spectra, Digital storage, Electric batteries, Mean square error, Capacity curves, Degradation predictions, Health status, Impedance spectrum, Partial voltage, Reliable operation, Safe operation, Forecasting
National Category
Other Electrical Engineering, Electronic Engineering, Information Engineering
Identifiers
URN: urn:nbn:se:mdh:diva-68071DOI: 10.1016/j.etran.2024.100347ISI: 001402993000001Scopus ID: 2-s2.0-85198007902OAI: oai:DiVA.org:mdh-68071DiVA, id: diva2:1884549
Available from: 2024-07-17 Created: 2024-07-17 Last updated: 2025-02-06Bibliographically approved

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Li, Hailong

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