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Deep neural network based battery impedance spectrum prediction using only impedance at characteristic frequencies
Joint Laboratory for Advanced Energy Storage and Application, School of Mechanical Engineering, Beijing Institute of Technology, No. 5 South Zhongguancun Street, Haidian District, Beijing, 100081, China.
Joint Laboratory for Advanced Energy Storage and Application, School of Mechanical Engineering, Beijing Institute of Technology, No. 5 South Zhongguancun Street, Haidian District, Beijing, 100081, China.
Joint Laboratory for Advanced Energy Storage and Application, School of Mechanical Engineering, Beijing Institute of Technology, No. 5 South Zhongguancun Street, Haidian District, Beijing, 100081, China.
Joint Laboratory for Advanced Energy Storage and Application, School of Mechanical Engineering, Beijing Institute of Technology, No. 5 South Zhongguancun Street, Haidian District, Beijing, 100081, China.
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2023 (English)In: Journal of Power Sources, ISSN 0378-7753, E-ISSN 1873-2755, Vol. 580, article id 233414Article in journal (Refereed) Published
Abstract [en]

Electrochemical impedance spectroscopy can be used for characterizing and monitoring the state of batteries. However, the difficulty in the onboard acquisition limits its wide applications. This work proposes a new method to obtain the impedance spectrum by using convolutional neural network, which uses the impedance measured at several characteristic frequencies as input. The characteristic frequencies are determined according to the time constants corresponding to the characteristic peaks and valleys of contact polarization and solid electrolyte interphase growth processes from the distribution of relaxation time. The proposed method is validated based on the dataset which contains the impedance spectra of eight batteries over the whole life cycle. The predictions coincide with the ground truth, with a maximum root mean square error of 0.93 mΩ. The developed method can also be quickly adapted to acquire the impedance spectrum of other batteries with different chemistries and be used for predictions of various battery states based on the transfer learning approach. 

Place, publisher, year, edition, pages
Elsevier B.V. , 2023. Vol. 580, article id 233414
Keywords [en]
Characteristic frequencies, Deep learning, Electrochemical impedance spectroscopy, Lithium-ion battery, Transfer learning, Convolutional neural networks, Deep neural networks, Forecasting, Life cycle, Lithium-ion batteries, Mean square error, Solid electrolytes, Battery impedance, Characteristic peaks, Characteristic-frequency, Convolutional neural network, Electrochemical-impedance spectroscopies, Impedance spectrum, Network-based, Time-constants
National Category
Other Electrical Engineering, Electronic Engineering, Information Engineering
Identifiers
URN: urn:nbn:se:mdh:diva-64015DOI: 10.1016/j.jpowsour.2023.233414ISI: 001048964800001Scopus ID: 2-s2.0-85165270646OAI: oai:DiVA.org:mdh-64015DiVA, id: diva2:1788554
Available from: 2023-08-16 Created: 2023-08-16 Last updated: 2023-08-30Bibliographically approved

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Li, Hailong

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